Ultrafast light wave electronics: Light from inside the tunnel

Date:
June 30, 2020
Source:
Forschungsverbund Berlin
Summary:
Steering and monitoring the light-driven motion of electrons
inside matter on the time-scale of a single optical cycle is a
key challenge in ultrafast light wave electronics and laser-based
material processing.

Physicists have now revealed a so-far overlooked nonlinear optical
mechanism that emerges from the light-induced tunneling of electrons
inside dielectrics.



FULL STORY ========================================================================== Steering and monitoring the light-driven motion of electrons
inside matter on the time-scale of a single optical cycle is a key
challenge in ultrafast light wave electronics and laser-based material processing. Physicists from the Max Born Institute in Berlin and the
University of Rostock have now revealed a so- far overlooked nonlinear
optical mechanism that emerges from the light-induced tunneling of
electrons inside dielectrics. For intensities near the material damage threshold, the nonlinear current arising during tunneling becomes
the dominant source of bright bursts of light, which are low-order
harmonics of the incident radiation. These findings, which have just been published in Nature Physics, significantly expand both the fundamental understanding of optical non-linearity in dielectric materials and its potential for applications in information processing and light-based
material processing.


==========================================================================
Our current understanding of non-linear optics at moderate light
intensities is based on the so-called Kerr non-linearity, which describes
the non-linear displacement of tightly bound electrons under the influence
of an incident optical light field. This picture changes dramatically
when the intensity of this light field is sufficiently high to eject
bound electrons from their ground state. At long wavelengths of the
incident light field, this scenario is associated with the phenomenon of tunneling, a quantum process where an electron performs a classically
forbidden transit through a barrier formed by the combined action of
the light force and the atomic potential.

Since the 1990's and pioneered by studies from the Canadian scientist
Franc,ois Brunel, the motion of electrons that have emerged at the
"end of the tunnel," which happens with maximal probability at the
crest of the light wave, has been considered as an important source for
optical non-linearity. This picture has now changed fundamentally. "In
the new experiment on glass, we could show that the current associated
with the quantum mechanical tunneling process itself creates an optical non-linearity that surpasses the traditional Brunel mechanism," explains
Dr. Alexandre Mermillod-Blondin from the Max Born Institute for Nonlinear Optics and Short Pulse Spectroscopy, who supervised the experiment. In
the experiment, two ultrashort light pulses with different wavelengths
and slightly different propagation directions were focused onto a thin
slab of glass, and a time- and frequency-resolved analysis of the emerging light emission was performed.

Identification of the mechanism responsible for this emission was
made possible by a theoretical analysis of the measurements that
was performed by the group of Prof. Thomas Fennel, who works at the
University of Rostock and at the Max Born Institute in the framework of
a DFG Heisenberg Professorship. "The analysis of the measured signals in
terms of a quantity that we termed the effective non-linearity was key
to distinguish the new ionization current mechanism from other possible mechanisms and to demonstrate its dominance," explains Fennel.

Future studies using this knowledge and the novel metrology method
that was developed in the course of this work may enable researchers to temporally resolve and steer strong-field ionization and avalanching in dielectric materials with unprecedented resolution, ultimately possibly
on the time-scale of a single cycle of light.


========================================================================== Story Source: Materials provided by Forschungsverbund_Berlin. Note:
Content may be edited for style and length.


========================================================================== Journal Reference:
1. P. Ju"rgens, B. Liewehr, B. Kruse, C. Peltz, D. Engel, A. Husakou,
T.

Witting, M. Ivanov, M. J. J. Vrakking, T. Fennel,
A. Mermillod-Blondin.

Origin of strong-field-induced low-order harmonic
generation in amorphous quartz. Nature Physics, 2020; DOI:
10.1038/s41567-020-0943-4 ==========================================================================

Link to news story: https://www.sciencedaily.com/releases/2020/06/200630111507.htm

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